optical spectroscopy of lanthanides magnetic and hyperfine interactions pdf

Optical Spectroscopy Of Lanthanides Magnetic And Hyperfine Interactions Pdf

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Optical Spectroscopy of Lanthanides in Crystalline Matrix

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The fundamental redox chemistry and valence electronic structure of the lanthanides in molecular complexes and extended solids continues to be a fertile area of research. The contemporary understanding of the accessible oxidation states of the lanthanide elements and the variability in their electronic structure is the result of several paradigm shifts. While the lanthanide elements have already found widespread use in technical and consumer applications, the continued reevaluation of basic redox properties is a central chemical concern to establish a more complete description of periodic properties. This fundamental understanding of valence electronic structure as it is derived from oxidation state and coordination environment is essential for the continued development of lanthanides in quantum information science and quantum materials research. This review presents the chemical and physical properties of tetravalent lanthanide ions in extended solids and molecules with a focus on the elements apart from cerium: praseodymium, neodymium, terbium, and dysprosium. If you are not the author of this article and you wish to reproduce material from it in a third party non-RSC publication you must formally request permission using Copyright Clearance Center. Go to our Instructions for using Copyright Clearance Center page for details.

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Optical Spectroscopy of Lanthanides

Systematics and the Properties of the Lanthanides pp Cite as. The energy level structure of free trivalent rare earth RE ions is discussed and its modification by the crystal field described. Modification of the crystal field spectra in imperfect crystals are discussed. Intensities and linewidth are considered. Finally divalent RE ions and magnetic interactions are mentioned briefly.


Optical Spectroscopy of Lanthanides: Magnetic and Hyperfine Interactions represents the sixth and final book by the late Brian Wybourne.


Optical Spectroscopy of Lanthanides in Crystalline Matrix

Notes on the Quantum Theory of Angular Momentum. Interactions in One- and Two-Electron Systems. Coupling Schemes of Angular Momenta. Magnetic Hyperfine Structure.

We outline first the simple theory of the magnetic hyperfine structure of an atom or ion in a state 4 f n , L, S, J , leaving the corrections which are generally small until later. Unable to display preview. Download preview PDF. Skip to main content.

Optical Spectroscopy of Lanthanides (eBook)

We outline first the simple theory of the magnetic hyperfine structure of an atom or ion in a state 4 f n , L, S, J , leaving the corrections which are generally small until later. Unable to display preview. Download preview PDF. Skip to main content.

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It then describes magnetic and hyperfine interactions and their impact on the energy structure and transition amplitudes of the lanthanide ions. The text culminates.


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